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Journal Articles

Evaluation on cementation by silicates in bentonite

Saito, Yuki*; Ishiwata, Tobimaru*; Horiuchi, Misato*; Nishiki, Yuto*; Kikuchi, Ryosuke*; Otake, Tsubasa*; Kawakita, Ryohei; Takayama, Yusuke; Mitsui, Seiichiro; Sato, Tsutomu*

Shigen, Sozai Koenshu (Internet), 11(1), 7 Pages, 2024/03

no abstracts in English

JAEA Reports

Acquisition of saltwater infiltration behavior data in unsaturated compacted bentonite

Sato, Hisashi*; Takayama, Yusuke; Suzuki, Hideaki*; Sato, Daisuke*

JAEA-Data/Code 2023-010, 47 Pages, 2023/09

JAEA-Data-Code-2023-010.pdf:1.45MB

When a high-level radioactive waste repository is constructed in a coastal area, it is necessary to fully evaluate the impact of seawater-based groundwater on engineered barriers, including buffer materials. In this report, one-dimensional saltwater infiltration tests were conducted to obtain data to understand the impact of seawater-based groundwater on the migration phenomena of water and solutes in the buffer material during the transient period. As a result, it was confirmed that the infiltration rate increased as the NaCl concentration in the infiltration solution increased. And it was confirmed that the water content ratio distribution changed as the NaCl concentration in the infiltration solution increased. As a result of analysis of the chloride ion concentration of the post-test specimens confirmed that chloride ion enrichment was occurred with infiltration. As a result of verifying the mechanism by which chloride ion enrichment occurs, it was confirmed that the phenomenon of chloride ion enrichment due to infiltration depends on the initial water content ratio.

Journal Articles

Secondary consolidation characteristic of bentonite by long-term consolidation tests of 2.7, 3.7 and 4 years

Takayama, Yusuke; Yamamoto, Yoichi*; Goto, Takahiro*

Jiban Kogaku Janaru (Internet), 18(3), p.317 - 330, 2023/09

It has been reported that the deformation greatly increased in the secondary consolidation process in the past long-term consolidation test of 1.8 years on Na-type bentonite/sand mixed soil. Therefore, we analyzed potential contributing factors in this behavior. A long-term consolidation test for about 10 years on bentonite and kaolinite was started using the test equipment with countermeasures against these factors. In this paper, the secondary consolidation behavior of bentonite was investigated based on the long-term consolidation test data for 2.7, 3.7 and 4 years. The results were generally consistent with the conventional findings on soil mechanics that the deformation due to secondary consolidation progresses linearly with respect to logarithm of time. This test will be continued for about 10 years and longer-term secondary consolidation behavior will be investigated.

Journal Articles

Proposition of confirmation items on the borehole sealing for the disposal of radioactive waste

Murakami, Hiroaki; Nishiyama, Nariaki; Takeuchi, Ryuji; Iwatsuki, Teruki

Oyo Chishitsu, 64(2), p.60 - 69, 2023/06

In order to confirm the quality control items for borehole closure in radioactive waste disposal projects, in-situ borehole sealing tests using bentonite material were conducted. As a result, the closure performance was successfully demonstrated by comparing the data of water injection tests conducted before and after the installation of the closure material. However, the breakthrough was observed after closing, probably due to high differential pressure applied to the seal section. Thus, it is important to ascertain throughout the entire operation that the borehole is adequately closed. The placement and specifications of the closure material should be determined according to the hydrogeological structure in the borehole. The confirmation items to use bentonite for sealing material are identified to be: to consider swelling and density loss in the borehole; to place the planned depth using appropriate emplacement technique; to be placed without damage to seals when use some backfilling materials, considering effect of permeability on adjacent seals.

Journal Articles

Effect of collapse behavior on changes in swelling pressure of bentonite during swelling pressure test

Takayama, Yusuke; Sato, Daisuke*; Kikuchi, Hirohito*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 29(2), p.101 - 111, 2022/12

Swelling pressure tests have been conducted to understand the swelling properties of bentonite which is planned to be used as a buffer material in repositories for the geological disposal of radioactive waste. It has been reported that the swelling pressure obtained by swelling pressure test increases monotonically or temporarily decreases after increasing with the passage of the time depending on the initial water content. In this study, swelling pressure tests were conducted under several different initial water content conditions, and the change in wet density distribution inside the specimen during the swelling pressure tests was observed by X-ray CT measurement. It was confirmed that the presence or absence of collapse behavior and its magnitude affect the shape of the change in swelling pressure. When the collapse deformation was large, the amount of temporary decrease in swelling pressure was large. On the other hand, swelling pressure increased monotonically when there was no deformation due to collapse.

JAEA Reports

Development of coupled mass-transport and chemical-reaction calculation code for alteration of engineered barrier

Sasagawa, Tsuyoshi; Mukai, Masayuki; Sawaguchi, Takuma

JAEA-Data/Code 2021-012, 122 Pages, 2022/01

JAEA-Data-Code-2021-012.pdf:3.87MB

Reducing public dose is required when radioactive wastes such as high-level and from reactor core internals etc. are disposed of by means of multi barrier system consist of engineered and natural barriers. In these barriers, engineered barrier is expected to bring out confinement function of waste's radionuclides in the barrier. Materials used as the engineered barriers are altered and performances of the barrier materials are degraded in course of time. To estimate properly the degraded performances, analytical evaluation of long-term change of the engineered barrier state is important. Change state of the engineered barrier is given by mass-transport and geochemical-reaction inside the barrier materials and these phenomena are interrelated, it is necessary to calculate the state by means of coupled analysis procedure. We have developed a coupled mass-transport and geochemical-reaction calculation code (MC- BUFFER) to evaluate alteration of engineered barrier specially targeted for water permeability of bentonite buffer material as one of most important performances to engineered barrier. This report describes functions expected for the engineered barrier, influence parameters for the functions, implementation models in MC-BUFFER, structure and functions of MC-BUFFER, input file format and output examples, execution method of MC-BUFFER, and sample run with MC-BUFFER.

Journal Articles

Observation of collapse behavior of bentonite during swelling pressure test using X-ray CT measurement

Takayama, Yusuke; Kikuchi, Hirohito*

Doboku Gakkai Rombunshu, C (Chiken Kogaku) (Internet), 77(3), p.302 - 313, 2021/09

Numerous swelling pressure tests have been conducted to understand the swelling properties of bentonite which is planned to be used as a buffer material in repositories for the geological disposal of radioactive waste. In this study, in order to clarify the cause of the decrease in swelling pressure during the swell-in pressure test period, the change in wet density distribution inside the specimen during the swelling pressure test was observed by X-ray CT measurement. It was supposed that this phenomenon was caused by the collapse inside the specimen. Furthermore, in order to confirm that collapse is generated by water absorption, the swelling deformation test was carried out under various load conditions. As a result, it was confirmed that collapse occurs even under the load conditions that are equal to or slightly smaller than the swelling pressure. These test data are expected to be used for validation of coupled analysis codes for evaluating the mechanical behavior of disposal facilities during re-saturation period.

Journal Articles

Commissioned research on geological disposal performed by JAEA Safety Research Center

Sawaguchi, Takuma

"Yugai Haikibutsu, Hoshasei Haikibutsu Eno Semento, Konkurito Gijutsu No Tekiyo Kenkyu Iinkai" Hokokusho (CD-ROM), p.165 - 173, 2020/12

no abstracts in English

Journal Articles

Impact of non-linear elastic behavior on bentonite density evolution at the FEBEX

Takayama, Yusuke

International Journal of Rock Mechanics and Mining Sciences, 136, p.104538_1 - 104538_8, 2020/12

 Times Cited Count:3 Percentile:25.28(Engineering, Geological)

It is necessary to apply reliable numerical simulation techniques to assess the mechanical behaviour of repositories for the geological disposal of radioactive waste over a long period of time. Having a constitutive model that can describe the mechanical behaviour of bentonite is key to such numerical simulations. In this study, the applicability of linear elastic constitutive model with swelling term is examined focusing on the density heterogeneity by applying to the in situ Full-scale Engineered Barrier Experiment (FEBEX) in Grimsel. It was confirmed that this constitutive model underestimates the density change. Instead, mechanical behaviour was re-simulated by unsaturated elasto-plastic constitutive model using the changes in degree of saturation as input data. Although no feedback effects of mechanical behaviour on hydraulic and thermal behaviour were taken into account, two-dimensional stress and density could be reproduced.

Journal Articles

Effect of water vapor on re-saturation process in EBS performance of re-saturation process by Thermo-Hydro-Mechanical coupled analysis

Sato, Shin*; Ono, Hirokazu; Tanai, Kenji; Yamamoto, Shuichi*; Fukaya, Masaaki*; Shimura, Tomoyuki*; Niunoya, Sumio*

Jiban Kogaku Janaru (Internet), 15(3), p.529 - 541, 2020/09

no abstracts in English

Journal Articles

A Study on applicability of elasto-plastic constitutive model to mechanical behavior of buffer material in salt water conditions

Takayama, Yusuke; Kikuchi, Hirohito*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 27(1), p.12 - 21, 2020/06

In this study, an applicability of the modified Cam clay model to the buffer material under saltwater conditions was examined. First, consolidated-undrained triaxial test was conducted using NaCl solution and artificial seawater. Based on the consolidated-undrained triaxial compression test results and the existing consolidation test results, the difference in the mechanical behavior of the buffer material under distilled water and saltwater condition was clarified. In particular, there was a difference in the unloading behavior in the consolidation test. Through reproducibility analysis of these experimental data, it was confirmed that the mechanical behavior of the buffer material can be roughly reproduced by setting the swelling index according to the salt concentration.

JAEA Reports

Backfilling test in drilling pits as part of Groundwater REcovery Experiment in Tunnel (GREET) Project

Takayasu, Kentaro; Onuki, Kenji*; Kawamoto, Koji*; Takayama, Yusuke; Mikake, Shinichiro; Sato, Toshinori; Onoe, Hironori; Takeuchi, Ryuji

JAEA-Technology 2017-011, 61 Pages, 2017/06

JAEA-Technology-2017-011.pdf:9.15MB

The Groundwater REcovery Experiment in Tunnel (GREET) was put into effect as development of drift backfilling technologies. This test was conducted by making the Closure Test Drift (CTD) recovered with water after carrying out a plug around 40m distance from northern edge face of horizontal tunnel of depth 500m, for the purpose of investigation of recovering process of rock mass and groundwater under the influence of excavation of tunnel. This report presents the efforts of backfilling investigation using bentonite composite soil and execution of backfilling into borehole pits excavated in the CTD which were carried out in fiscal 2014 as a part of GREET, and succeeding observation results inside pits from September 2014 to March 2016.

Journal Articles

Long-term mechanical analysis code considering chemical alteration for a TRU waste geological repository

Mihara, Morihiro; Hirano, Fumio; Takayama, Yusuke; Kyokawa, Hiroyuki*; Ono, Shintaro*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 24(1), p.15 - 25, 2017/06

A computer program MACBECE has been developed to provide rigorous calculations of the long-term mechanical behavior of a TRU waste geological repository. Consideration is given to the expected chemical alteration of repository components, including cementitious materials and bentonite, and the mechanical interactions between repository and host rock. The long-term mechanical behavior of a TRU waste repository was evaluated in a deep soft rock site, where creep deformation is likely to occur from the initial construction phase to 10$$^{5}$$ years after repository closure. It was found that the stress didn't fall into a singularity of yield surface of the EC model applied to the mechanical behavior model of bentonite. The calculated displacement of the inner diameter of the repository, considering mechanical interaction between repository and host rock, was about half that of a result in 2nd progress report on R&D for TRU waste disposal in Japan.

JAEA Reports

Environmental remediation for the upstream of Yotsugi Mill Tailings Pond, Ningyo-toge Uranium Mine

Saito, Hiroshi; Sato, Yasushi*; Sakamoto, Atsushi*; Torikai, Kazuyoshi; Fukushima, Shigeru; Sakao, Ryota; Taki, Tomihiro

JAEA-Technology 2015-063, 119 Pages, 2016/03

JAEA-Technology-2015-063.pdf:86.2MB

Ningyo-toge Environmental Engineering Center has been conducting environmental remediation of the Ningyo-toge Uranium Mine, after decades of mine-related activities were terminated. Its purposes are to take measures to ensure safety and radiation protection from the exposure pathways to humans in future, and to prevent the occurrence of mining pollution. As part of the remediation, upstream part of the Yotsugi Mill Tailings Pond, the highest prioritized facility, has been remediated to fiscal year 2012. Multi-layered capping has been constructed using natural material, after specifications and whole procedure being examined in terms of long-term stability, radiation protection, economics, etc. Monitoring has been carried out to confirm the effectiveness of the capping, in terms of settlement, dose and radon exhalation rates, etc. Monitoring of drainage volume of penetrated rainwater is planned. Accumulated data will be examined and used for remediation of downstream part of the Pond.

Journal Articles

Evaluation of uncertainty associated with parameters for long-term safety assessments of geological disposal

Yamaguchi, Tetsuji; Minase, Naofumi; Iida, Yoshihisa; Tanaka, Tadao; Nakayama, Shinichi

JAERI-Conf 2005-007, p.150 - 155, 2005/08

no abstracts in English

Journal Articles

Long-term alteration of bentonite; For safety evaluation of deep geological disposal

Tanaka, Tadao; Sakamoto, Yoshifumi; Yamaguchi, Tetsuji; Takazawa, Mayumi; Akai, Masanobu; Negishi, Kumi; Iida, Yoshihisa; Nakayama, Shinichi

JAERI-Conf 2005-007, p.105 - 110, 2005/08

Highly alkaline environments induced by cementitious materials in radioactive waste repositories are likely to dissolve and to alter montmorillonite, the main constituent of bentonite buffer materials. For the prediction of the long-term variations in permeability of compacted sand-bentonite mixtures, long-term alteration of bentonite should be quantified based on information accumulated by using the compacted or powdered bentonite materials, with batch experiments or column experiments. In this study, we summarize distinctive information obtained from various experimental systems, and propose functional and effective integration of experimental approaches to prediction of bentonite alteration.

Journal Articles

Experimental and modeling study to predict long-term alteration of bentonite buffer materials with alkaline groundwater

Takazawa, Mayumi; Negishi, Kumi; Sakamoto, Yoshifumi; Akai, Masanobu; Yamaguchi, Tetsuji; Iida, Yoshihisa; Tanaka, Tadao; Nakayama, Shinichi

JAERI-Conf 2005-007, p.236 - 241, 2005/08

no abstracts in English

Journal Articles

Modeling of variation in permeability of compacted bentonite with alkaline fluid for long-term safety assessment of geological disposal system

Takazawa, Mayumi; Yamaguchi, Tetsuji; Sakamoto, Yoshifumi; Akai, Masanobu; Tanaka, Tadao; Nakayama, Shinichi

NUMO-TR-04-05, p.A3_59 - A3_62, 2004/10

no abstracts in English

Journal Articles

Field tests on migration of TRU-nuclide, 2; Migration test for engineered barrier materials in aerated soil

Maeda, Toshikatsu; Tanaka, Tadao; Mukai, Masayuki; Ogawa, Hiromichi; Yamaguchi, Tetsuji; Munakata, Masahiro; Matsumoto, Junko; Kozai, Naofumi; Bamba, Tsunetaka; Fan, Z.*; et al.

Nihon Genshiryoku Gakkai Wabun Rombunshi, 2(3), p.336 - 341, 2003/09

no abstracts in English

JAEA Reports

Activation energy of diffusivities for deuterated water in compacted sodium-bentonite; Through-diffusion experiment and molecular dynamics simulation

Suzuki, Satoru; Sato, Haruo; Ishidera, Takamitsu; Fujii, Naoki*; Kawamura, Katsuyuki*

JNC TN8400 2001-031, 44 Pages, 2002/05

JNC-TN8400-2001-031.pdf:1.58MB

In order to quantify effect of temperature on diffusivity of deuterated water (HDO) in compacted sodium-bentonite, through-diffusion experiments were conducted at elevated tempemture from 298 to 333 K. Kunipia F (Na-montmorillonite content $$>$$ 98 wt. %; Kunimine Industly Co.) was compacted to a dry density of 0.9 and l.35 Mg/m$$^{3}$$. Since smectite flakes were perpendicularly oriented to a direction of compaction, anisotropy of diffusivity was investigated parallel and normal to the preferred orientation of smectite. Effective diffusion coeficient D$$_{e}$$ of HDO was larger for a diffusional direction parallel to the preferred orientation than normal to that for both dry densities. These results well agreed to the previously reported ones for tritiated water. Activation energies of D$$_{e}$$ in compacted bentonite increased with increasing dry density in the range of 19 - 25 kJ/mol which was slightly larger than that in bulk water (18 kJ/mol). This relationship can be considered to be due to both the pore structure development and high activation energy of water (18-23 kJ/mol) in the vicinity of smectite surface (within 2 nm) on the basis of molecular dynamics simulations.

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